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DESCRIPTION:The assembly of van der Waals heterostructures enables the crea
 tion of devices comprising materials with vastly different electronic band
  structures\, overcoming the limitations of matching crystal structures. S
 andwiching an insulator between two (semi-)metallic electrodes constitutes
  a blueprint for a rational design of tunnelling devices\, where bidirecti
 onal injection of electrons and holes onto the radiative states leads to e
 lectroluminescent processes. The nature of the radiative states may be vas
 tly different\, including Wannier-Mott-like excitons in semiconductors [1\
 ,2]\, Frenkel excitons coupled to magnetization textures in ferromagnets [
 3\,4]\, or intradefect transitions raising single photons [5-9]. The struc
 ture of the barrier can be complex\, involving multiple materials with ato
 mically precise thickness. Consequently\, the efficiency of the electrolum
 inescent processes is tunable across multiple orders of magnitude due to t
 he competition between the tunnelling dynamics and the radiative lifetimes
 . Alternative tunnelling pathways are activated by distinct device archite
 ctures at the material level\, governing their spectroscopic characteristi
 cs.\n\nReferences\n\n[1] K. Walczyk\, G. Krasucki\, K. Olkowska-Pucko\, Z.
  Chen\, T. Taniguchi\, K. Watanabe\, A. Babiński\, M. Koperski\, M. R. Mo
 las\, N. Zawadzka\, Optical response of WSe2-based vertical tunneling junc
 tion\, Solid State Communications 396\, 115756 (2025).\n\n[2] J. Zultak\, 
 S. J. Magorrian\, M. Koperski\, A. Garner\, M. J. Hamer\, E. Tóvári\, K.
  S. Novoselov\, A. A. Zhukov\, Y. Zou\, N. R. Wilson\, S. J. Haigh\, A. V.
  Kretinin\, V. I Fal’ko\, R. Gorbachev\, Ultra-thin van der Waals crysta
 ls as semiconductor quantum wells\, Nature Communications 11 (1)\, 125 (20
 20).\n\n[3] M. Grzeszczyk\, S. Acharya\, D. Pashov\, Z. Chen\, K. Vaklinov
 a\, M. van Schilfgaarde\, K. Watanabe\, T. Taniguchi\, K. S. Novoselov\, M
 . I. Katsnelson\, M. Koperski\, Strongly Correlated Exciton‐Magnetizatio
 n System for Optical Spin Pumping in CrBr3 and CrI3\, Advanced Materials 3
 5 (17)\, 2209513 (2023).\n\n[4] S. Grebenchuk\, C. McKeever\, M. Grzeszczy
 k\, Z. Chen\, M. Šiškins\, A. R. C. McCray\, Y. Li\, A. K. Petford‐Lon
 g\, C. M. Phatak\, D. Ruihuan\, L. Zheng\, K. S. Novoselov\, E. J. G. Sant
 os\, M. Koperski\, Topological spin textures in an insulating van der Waal
 s ferromagnet\, Advanced Materials 36 (24)\, 2311949 (2024).\n\n[5] M. Grz
 eszczyk\, K. Vaklinova\, K. Watanabe\, T. Taniguchi\, K. S. Novoselov\, M.
  Koperski\, Electroluminescence from pure resonant states in hBN-based ver
 tical tunneling junctions\, Light: Science &amp; Applications 13 (1)\, 155 (20
 24).\n\n[6] J. Howarth\, K. Vaklinova\, M. Grzeszczyk\, G. Baldi\, L. Hagu
 e\, M. Potemski\, K. S. Novoselov\, A. Kozikov\, M. Koperski\, PNAS 121 (2
 3)\, e2401757121 (2024).\n\n[7] Z. Qiu\, K. Vaklinova\, P. Huang\, M. Grze
 szczyk\, K. Watanabe\, T. Taniguchi\, K. S. Novoselov\, J. Lu\, M. Kopersk
 i\, Atomic and Electronic Structure of Defects in hBN: Enhancing Single-De
 fect Functionalities\, ACS Nano 18 (35)\, 24035–24043 (2024).\n\n[8] L. 
 Loh\, J. Wang\, M. Grzeszczyk\, M. Koperski\, G. Eda\, Towards quantum lig
 ht-emitting devices based on van der Waals materials\, Nature Reviews Elec
 trical Engineering 1\, 815–829 (2024).\n\n[9] D. Litvinov\, A. Wu\, M. B
 arbosa\, K. Vaklinova\, M. Grzeszczyk\, G. Baldi\, M. Zhu\, M. Koperski\, 
 Single photon sources and single electron transistors in two-dimensional m
 aterials\, Materials Science and Engineering: R: Reports 163\, 100928 (202
 5).\n\nSpeaker(s): \, Maciej Koperski\n\nVirtual: https://events.vtools.ie
 ee.org/m/495090
LOCATION:Virtual: https://events.vtools.ieee.org/m/495090
ORGANIZER:cd@anl.gov
SEQUENCE:5
SUMMARY:Electron tunnelling in vertical van der Waals junctions for electro
 luminescent devices
URL;VALUE=URI:https://events.vtools.ieee.org/m/495090
X-ALT-DESC:Description: &lt;br /&gt;&lt;p class=&quot;MsoNormal&quot;&gt;The assembly of van der 
 Waals heterostructures enables the creation of devices comprising material
 s with vastly different electronic band structures\, overcoming the limita
 tions of matching crystal structures. Sandwiching an insulator between two
  (semi-)metallic electrodes constitutes a blueprint for a rational design 
 of tunnelling devices\, where bidirectional injection of electrons and hol
 es onto the radiative states leads to electroluminescent processes. The na
 ture of the radiative states may be vastly different\, including Wannier-M
 ott-like excitons in semiconductors &lt;strong&gt;[1\,2]&lt;/strong&gt;\, Frenkel exci
 tons coupled to magnetization textures in ferromagnets &lt;strong&gt;[3\,4]&lt;/str
 ong&gt;\, or intradefect transitions raising single photons &lt;strong&gt;[5-9]&lt;/st
 rong&gt;. The structure of the barrier can be complex\, involving multiple ma
 terials with atomically precise thickness. Consequently\, the efficiency o
 f the electroluminescent processes is tunable across multiple orders of ma
 gnitude due to the competition between the tunnelling dynamics and the rad
 iative lifetimes. Alternative tunnelling pathways are activated by distinc
 t device architectures at the material level\, governing their spectroscop
 ic characteristics.&lt;/p&gt;\n&lt;p class=&quot;MsoNormal&quot;&gt;&amp;nbsp\;&lt;/p&gt;\n&lt;p class=&quot;MsoNo
 rmal&quot;&gt;&lt;strong&gt;References&lt;/strong&gt;&lt;/p&gt;\n&lt;p class=&quot;MsoNormal&quot;&gt;[1] K. Walczyk
 \, G. Krasucki\, K. Olkowska-Pucko\, Z. Chen\, T. Taniguchi\, K. Watanabe\
 , A. Babiński\, M. Koperski\, M. R. Molas\, N. Zawadzka\, &lt;em&gt;Optical res
 ponse of WSe&lt;sub&gt;2&lt;/sub&gt;-based vertical tunneling junction&lt;/em&gt;\, Solid St
 ate Communications &lt;strong&gt;396&lt;/strong&gt;\, 115756 (2025).&lt;/p&gt;\n&lt;p class=&quot;Ms
 oNormal&quot;&gt;[2] J. Zultak\, S. J. Magorrian\, M. Koperski\, A. Garner\, M. J.
  Hamer\, E. T&amp;oacute\;v&amp;aacute\;ri\, K. S. Novoselov\, A. A. Zhukov\, Y. Z
 ou\, N. R. Wilson\, S. J. Haigh\, A. V. Kretinin\, V. I Fal&amp;rsquo\;ko\, R.
  Gorbachev\, &lt;em&gt;Ultra-thin van der Waals crystals as semiconductor quantu
 m wells&lt;/em&gt;\, Nature Communications &lt;strong&gt;11 (1)&lt;/strong&gt;\, 125 (2020).
 &lt;/p&gt;\n&lt;p class=&quot;MsoNormal&quot;&gt;[3] M. Grzeszczyk\, S. Acharya\, D. Pashov\, Z.
  Chen\, K. Vaklinova\, M. van Schilfgaarde\, K. Watanabe\, T. Taniguchi\, 
 K. S. Novoselov\, M. I. Katsnelson\, M. Koperski\, &lt;em&gt;Strongly Correlated
  Exciton‐Magnetization System for Optical Spin Pumping in CrBr&lt;sub&gt;3&lt;/su
 b&gt; and CrI&lt;sub&gt;3&lt;/sub&gt;&lt;/em&gt;\, Advanced Materials &lt;strong&gt;35 (17)&lt;/strong&gt;\
 , 2209513 (2023).&lt;/p&gt;\n&lt;p class=&quot;MsoNormal&quot;&gt;[4] S. Grebenchuk\, C. McKeeve
 r\, M. Grzeszczyk\, Z. Chen\, M. &amp;Scaron\;i&amp;scaron\;kins\, A. R. C. McCray
 \, Y. Li\, A.&amp;nbsp\;K.&amp;nbsp\;Petford‐Long\, C. M. Phatak\, D. Ruihuan\, 
 L. Zheng\, K. S. Novoselov\, E. J. G. Santos\, M.&amp;nbsp\;Koperski\, &lt;em&gt;Top
 ological spin textures in an insulating van der Waals ferromagnet&lt;/em&gt;\, A
 dvanced Materials &lt;strong&gt;36 (24)&lt;/strong&gt;\, 2311949 (2024).&lt;/p&gt;\n&lt;p class
 =&quot;MsoNormal&quot;&gt;[5] M. Grzeszczyk\, K. Vaklinova\, K. Watanabe\, T. Taniguchi
 \, K. S. Novoselov\, M. Koperski\, &lt;em&gt;Electroluminescence from pure reson
 ant states in hBN-based vertical tunneling junctions&lt;/em&gt;\, Light: Science
  &amp;amp\; Applications &lt;strong&gt;13 (1)&lt;/strong&gt;\, 155 (2024).&lt;/p&gt;\n&lt;p class=&quot;
 MsoNormal&quot;&gt;[6] J. Howarth\, K. Vaklinova\, M. Grzeszczyk\, G. Baldi\, L. H
 ague\, M. Potemski\, K. S. Novoselov\, A.&amp;nbsp\;Kozikov\, M. Koperski\, PN
 AS &lt;strong&gt;121 (23)&lt;/strong&gt;\, e2401757121 (2024).&lt;/p&gt;\n&lt;p class=&quot;MsoNorma
 l&quot;&gt;[7] Z. Qiu\, K. Vaklinova\, P. Huang\, M. Grzeszczyk\, K. Watanabe\, T.
  Taniguchi\, K. S. Novoselov\, J. Lu\, M. Koperski\, &lt;em&gt;Atomic and Electr
 onic Structure of Defects in hBN: Enhancing Single-Defect Functionalities&lt;
 /em&gt;\, ACS Nano &lt;strong&gt;18 (35)&lt;/strong&gt;\, 24035&amp;ndash\;24043 (2024).&lt;/p&gt;\
 n&lt;p class=&quot;MsoNormal&quot;&gt;[8] L. Loh\, J. Wang\, M. Grzeszczyk\, M. Koperski\,
  G. Eda\, &lt;em&gt;Towards quantum light-emitting devices based on van der Waal
 s materials&lt;/em&gt;\, Nature Reviews Electrical Engineering &lt;strong&gt;1&lt;/strong
 &gt;\, 815&amp;ndash\;829 (2024).&lt;/p&gt;\n&lt;p class=&quot;MsoNormal&quot;&gt;[9] D. Litvinov\, A. 
 Wu\, M. Barbosa\, K. Vaklinova\, M. Grzeszczyk\, G. Baldi\, M. Zhu\, M. Ko
 perski\, &lt;em&gt;Single photon sources and single electron transistors in two-
 dimensional materials&lt;/em&gt;\, Materials Science and Engineering: R: Reports
  &lt;strong&gt;163&lt;/strong&gt;\, 100928 (2025).&lt;/p&gt;
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